Tricyclic analogues of epidithiodioxopiperazine alkaloids with promising in vitro and in vivo antitumor activity

نویسندگان

  • Marcus Baumann
  • André P. Dieskau
  • Brad M. Loertscher
  • Mary C. Walton
  • Sangkil Nam
  • Jun Xie
  • David Horne
  • Larry E. Overman
چکیده

Department of Chemistry, 1102 Natural Sc California 92697-2025, USA. E-mail: leoverm Department of Molecular Medicine, Bec Comprehensive Cancer Center, 1500 E. D USA. E-mail: [email protected] † Electronic supplementary information (E and diastereoselectivity in the synthesis of procedures, and characterization data 1061869–1061873. For ESI and crystallog format see DOI: 10.1039/c5sc01536g Cite this: Chem. Sci., 2015, 6, 4451

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Tricyclic analogues of epidithiodioxopiperazine alkaloids with promising in vitro and in vivo antitumor activity† †Electronic supplementary information (ESI) available: Table summarizing yields and diastereoselectivity in the synthesis of ETP alkaloid analogues 3, experimental procedures, and characterization data for all new compounds. CCDC 1061869–1061873. For ESI and crystallographic data in CIF or other electronic format see DOI: 10.1039/c5sc01536g Click here for additional data file. Click here for additional data file.

Epipolythiodioxopiperazine (ETP) alkaloids are structurally elaborate alkaloids that show potent antitumor activity. However, their high toxicity and demonstrated interactions with various biological receptors compromises their therapeutic potential. In an effort to mitigate these disadvantages, a short stereocontrolled construction of tricyclic analogues of epidithiodioxopiperazine alkaloids w...

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تاریخ انتشار 2015